Ultrafast electron diffraction: Visualizing dynamic states of matter

D Filippetto, P Musumeci, RK Li, BJ Siwick… - Reviews of Modern …, 2022 - APS
Since the discovery of electron-wave duality, electron scattering instrumentation has
developed into a powerful array of techniques for revealing the atomic structure of matter …

Brighter, faster, stronger: ultrafast scattering of free molecules

A Odate, A Kirrander, PM Weber… - Advances in Physics …, 2023 - Taylor & Francis
Advances in FEL technologies have contributed remarkably to various scientific fields over
the past decade, and ultrafast molecular dynamics is no exception. The ability to probe …

Simultaneous observation of nuclear and electronic dynamics by ultrafast electron diffraction

J Yang, X Zhu, JP F. Nunes, JK Yu, RM Parrish… - Science, 2020 - science.org
Simultaneous observation of nuclear and electronic motion is crucial for a complete
understanding of molecular dynamics in excited electronic states. It is challenging for a …

Femtosecond electronic and hydrogen structural dynamics in ammonia imaged with ultrafast electron diffraction

EG Champenois, NH List, M Ware, M Britton… - Physical Review Letters, 2023 - APS
Directly imaging structural dynamics involving hydrogen atoms by ultrafast diffraction
methods is complicated by their low scattering cross sections. Here we demonstrate that …

Monitoring the evolution of relative product populations at early times during a photochemical reaction

JP Figueira Nunes, LM Ibele, S Pathak… - Journal of the …, 2024 - ACS Publications
Identifying multiple rival reaction products and transient species formed during ultrafast
photochemical reactions and determining their time-evolving relative populations are key …

Conformer-specific photochemistry imaged in real space and time

EG Champenois, DM Sanchez, J Yang… - Science, 2021 - science.org
Conformational isomers (conformers) of molecules play a decisive role in biology and
organic chemistry. However, experimental methods for investigating chemical reaction …

UV-Induced Reaction Pathways in Bromoform Probed with Ultrafast Electron Diffraction

L Hoffmann, BW Toulson, J Yang… - Journal of the …, 2024 - ACS Publications
For many chemical reactions, it remains notoriously difficult to predict and experimentally
determine the rates and branching ratios between different reaction channels. This is …

[HTML][HTML] Relativistic ultrafast electron diffraction at high repetition rates

KM Siddiqui, DB Durham, F Cropp, F Ji… - Structural …, 2023 - pubs.aip.org
The ability to resolve the dynamics of matter on its native temporal and spatial scales
constitutes a key challenge and convergent theme across chemistry, biology, and materials …

Molecular structure retrieval directly from laboratory-frame photoelectron spectra in laser-induced electron diffraction

A Sánchez, K Amini, SJ Wang, T Steinle… - Nature …, 2021 - nature.com
Ubiquitous to most molecular scattering methods is the challenge to retrieve bond distance
and angle from the scattering signals since this requires convergence of pattern matching …

High-resolution movies of molecular rotational dynamics captured with ultrafast electron diffraction

Y Xiong, KJ Wilkin, M Centurion - Physical Review Research, 2020 - APS
Imaging the structure of molecules during a photoinduced reaction is essential for
elucidating reaction mechanisms. This requires high spatiotemporal resolution to capture …