Quantum design of photosynthesis for bio-inspired solar-energy conversion

E Romero, VI Novoderezhkin, R Van Grondelle - Nature, 2017 - nature.com
Photosynthesis is the natural process that converts solar photons into energy-rich products
that are needed to drive the biochemistry of life. Two ultrafast processes form the basis of …

Photosynthetic light-harvesting (antenna) complexes—structures and functions

H Lokstein, G Renger, JP Götze - Molecules, 2021 - mdpi.com
Chlorophylls and bacteriochlorophylls, together with carotenoids, serve, noncovalently
bound to specific apoproteins, as principal light-harvesting and energy-transforming …

Photochemistry beyond the red limit in chlorophyll f–containing photosystems

DJ Nürnberg, J Morton, S Santabarbara, A Telfer… - Science, 2018 - science.org
Photosystems I and II convert solar energy into the chemical energy that powers life.
Chlorophyll a photochemistry, using red light (680 to 700 nm), is near universal and is …

Accurate Computation of the Absorption Spectrum of Chlorophyll a with Pair Natural Orbital Coupled Cluster Methods

A Sirohiwal, R Berraud-Pache, F Neese… - The Journal of …, 2020 - ACS Publications
The ability to accurately compute low-energy excited states of chlorophylls is critically
important for understanding the vital roles they play in light harvesting, energy transfer, and …

Protein matrix control of reaction center excitation in photosystem II

A Sirohiwal, F Neese, DA Pantazis - Journal of the American …, 2020 - ACS Publications
Photosystem II (PSII) is a multisubunit pigment–protein complex that uses light-induced
charge separation to power oxygenic photosynthesis. Its reaction center chromophores …

Quasiparticle Self-Consistent GW-Bethe–Salpeter Equation Calculations for Large Chromophoric Systems

A Förster, L Visscher - Journal of chemical theory and …, 2022 - ACS Publications
The GW-Bethe–Salpeter equation (BSE) method is promising for calculating the low-lying
excitonic states of molecular systems. However, so far it has only been applied to rather …

Tuning the intrinsic properties of carbon nitride for high quantum yield photocatalytic hydrogen production

MZ Rahman, K Davey, CB Mullins - Advanced Science, 2018 - Wiley Online Library
The low quantum yield of photocatalytic hydrogen production in carbon nitride (CN) has
been improved upon via the modulation of both the extrinsic and intrinsic properties of the …

Advances in the spectroscopic and structural characterization of core light-harvesting complexes from purple phototrophic bacteria

Y Kimura, K Tani, MT Madigan… - The Journal of Physical …, 2023 - ACS Publications
Purple phototrophic bacteria are ancient anoxygenic phototrophs and attractive research
tools because they capture light energy in the near-infrared (NIR) region of the spectrum and …

Structural basis of light‐harvesting in the photosystem II core complex

F Müh, A Zouni - Protein Science, 2020 - Wiley Online Library
Photosystem II (PSII) is a membrane‐spanning, multi‐subunit pigment–protein complex
responsible for the oxidation of water and the reduction of plastoquinone in oxygenic …

Vibronic structure of photosynthetic pigments probed by polarized two-dimensional electronic spectroscopy and ab initio calculations

Y Song, A Schubert, E Maret, RK Burdick… - Chemical …, 2019 - pubs.rsc.org
Bacteriochlorophyll a (Bchl a) and chlorophyll a (Chl a) play important roles as light
absorbers in photosynthetic antennae and participate in the initial charge-separation steps …