Nitrogen fixation via splitting into nitrido complexes

SJK Forrest, B Schluschaß, EY Yuzik-Klimova… - Chemical …, 2021 - ACS Publications
The large carbon footprint of the Haber–Bosch process, which provides ammonia for
fertilizers but also the feedstock for all nitrogenous commercial products, has fueled the …

Activation of dinitrogen by polynuclear metal complexes

D Singh, WR Buratto, JF Torres, LJ Murray - Chemical reviews, 2020 - ACS Publications
Activation of dinitrogen plays an important role in daily anthropogenic life, and the processes
by which this fixation occurs have been a longstanding and significant research focus within …

Breaking scaling relations to achieve low-temperature ammonia synthesis through LiH-mediated nitrogen transfer and hydrogenation

P Wang, F Chang, W Gao, J Guo, G Wu, T He… - Nature chemistry, 2017 - nature.com
Ammonia synthesis under mild conditions is a goal that has been long sought after. Previous
investigations have shown that adsorption and transition-state energies of intermediates in …

Nickel hydride complexes

NA Eberhardt, H Guan - Chemical reviews, 2016 - ACS Publications
Nickel hydride complexes, defined herein as any molecules bearing a nickel hydrogen
bond, are crucial intermediates in numerous nickel-catalyzed reactions. Some of them are …

Complexes of Ni (I): a “rare” oxidation state of growing importance

CY Lin, PP Power - Chemical Society Reviews, 2017 - pubs.rsc.org
Nickel plays an important role in areas as diverse as metallurgy, magnetism and biology as
well as in chemical applications such as the catalytic transformation of organic substrates …

The chemistry of univalent metal β-diketiminates

YC Tsai - Coordination Chemistry Reviews, 2012 - Elsevier
The easily electronically and sterically tunable β-diketiminates are widely used auxiliary
ligands for the creation of a wide range of metal complexes with various oxidation states in …

Metal–dioxygen and metal–dinitrogen complexes: where are the electrons?

PL Holland - Dalton transactions, 2010 - pubs.rsc.org
Transition-metal complexes of O2 and N2 play an important role in the environment,
chemical industry, and metalloenzymes. This Perspective compares and contrasts the …

Ni (I)–X complexes bearing a bulky α-diimine ligand: synthesis, structure, and superior catalytic performance in the hydrogen isotope exchange in pharmaceuticals

C Zarate, H Yang, MJ Bezdek, D Hesk… - Journal of the American …, 2019 - ACS Publications
The synthesis and spectroscopic characterization of a family of Ni–X (X= Cl, Br, I, H)
complexes supported by the bulky α-diimine chelate N, N′-bis (1 R, 2 R, 3 R, 5 S)-(−) …

Donor‐Acceptor Activation of Carbon Dioxide

M Pérez‐Jiménez, H Corona… - … A European Journal, 2023 - Wiley Online Library
The activation and functionalization of carbon dioxide entails great interest related to its
abundance, low toxicity and associated environmental problems. However, the inertness of …

A d10 Ni–(H2) Adduct as an Intermediate in HH Oxidative Addition across a NiB Bond

WH Harman, TP Lin, JC Peters - … Chemie International Edition, 2014 - Wiley Online Library
Abstract Bifunctional E H activation offers a promising approach for the design of two‐
electron‐reduction catalysts with late first‐row metals, such as Ni. To this end, we have been …