Recent advances in polysaccharide-based self-healing hydrogels for biomedical applications

Y Yang, L Xu, J Wang, Q Meng, S Zhong, Y Gao… - Carbohydrate …, 2022 - Elsevier
Hydrogels are a class of polymer materials with three-dimensional networks structure, which
can absorb a large number of water and biological fluids. Natural polysaccharides are ideal …

Designing hydrogels for 3D cell culture using dynamic covalent crosslinking

M Rizwan, AEG Baker… - Advanced Healthcare …, 2021 - Wiley Online Library
Designing simple biomaterials to replicate the biochemical and mechanical properties of
tissues is an ongoing challenge in tissue engineering. For several decades, new …

Disulfide-mediated reversible polymerization toward intrinsically dynamic smart materials

Q Zhang, DH Qu, BL Feringa… - Journal of the American …, 2022 - ACS Publications
The development of a dynamic chemistry toolbox to endow materials dynamic behavior has
been key to the rational design of future smart materials. The rise of supramolecular and …

Self-healing polyurethane with high strength and toughness based on a dynamic chemical strategy

F Dong, X Yang, L Guo, Y Wang… - Journal of Materials …, 2022 - pubs.rsc.org
The introduction of disulfide bonds in polyurethane elastomers confers self-healing and
recyclable properties to the elastomers, which not only reduce the maintenance cost but also …

Preparation of non-isocyanate polyurethanes from epoxy soybean oil: dual dynamic networks to realize self-healing and reprocessing under mild conditions

X Yang, S Wang, X Liu, Z Huang, X Huang, X Xu… - Green …, 2021 - pubs.rsc.org
Non-isocyanate polyurethanes prepared using cyclic carbonates derived from epoxy
soybean oil and CO2 can exhibit the reprocessing ability and facilitate the realization of …

Acid‐catalyzed Disulfide‐mediated Reversible Polymerization for Recyclable Dynamic Covalent Materials

BS Wang, Q Zhang, ZQ Wang, CY Shi… - Angewandte Chemie …, 2023 - Wiley Online Library
Abstract Poly (1, 2‐dithiolane) s are a family of intrinsically recyclable polymers due to their
dynamic covalent disulfide linkages. Despite the common use of thiolate‐initiated anionic …

Light-mediated synthesis and reprocessing of dynamic bottlebrush elastomers under ambient conditions

C Choi, JL Self, Y Okayama, AE Levi… - Journal of the …, 2021 - ACS Publications
We introduce a novel grafting-through polymerization strategy to synthesize dynamic
bottlebrush polymers and elastomers in one step using light to construct a disulfide …

Photoinduced dithiolane crosslinking for multiresponsive dynamic hydrogels

BR Nelson, BE Kirkpatrick, CE Miksch… - Advanced …, 2023 - Wiley Online Library
While many hydrogels are elastic networks crosslinked by covalent bonds, viscoelastic
hydrogels with adaptable crosslinks are increasingly being developed to better recapitulate …

Dual closed-loop chemical recycling of synthetic polymers by intrinsically reconfigurable poly (disulfides)

Q Zhang, Y Deng, CY Shi, BL Feringa, H Tian, DH Qu - Matter, 2021 - cell.com
The excessive use of plastics has led to severe global problems involving environmental,
energy, and health issues and demands for sustainable and recyclable alternatives. Toward …

Molecularly engineered cardanol derived epoxy vitrimers based on dynamic disulfide and dynamic ester exchanges with desirable dynamic response, degradability …

Y Hu, S Tong, L Hu, M Zhang, Q Huang, Y Sha… - Chemical Engineering …, 2023 - Elsevier
Dynamic covalent chemistry provides a solution to the recycling problem of epoxy resins,
and the graphene functional composites. Nevertheless, the study on chemical structures of …